The rotational motion of an iSN nitroxide in diisobutylphthalate solutions at varied temperatures has been studied for correlation times from 1Om8 to > 10m3 sec. Data from both conventional (first-harmonic, in-phase) and saturation-transfer (second-harmonic, out-of-phase) EPR are reported. For many spectral parameters, including linewidth, position of outer extrema, and ratios of spectral ampli...