نتایج جستجو برای: exciton binding energy

تعداد نتایج: 1067675  

2017
Noritake Murakami Yuto Tango Hideaki Miyake Tomoyuki Tajima Yuta Nishina Wataru Kurashige Yuichi Negishi Yutaka Takaguchi

Single-walled carbon nanotubes (SWCNTs) are potentially strong optical absorbers with tunable absorption bands depending on their chiral indices (n, m). Their application for solar energy conversion is difficult because of the large binding energy (>100 meV) of electron-hole pairs, known as excitons, produced by optical absorption. Recent development of photovoltaic devices based on SWCNTs as l...

Journal: :The journal of physical chemistry letters 2014
Tom J Savenije Carlito S Ponseca Lucas Kunneman Mohamed Abdellah Kaibo Zheng Yuxi Tian Qiushi Zhu Sophie E Canton Ivan G Scheblykin Tonu Pullerits Arkady Yartsev Villy Sundström

Solar cells based on organometal halide perovskites have seen rapidly increasing efficiencies, now exceeding 15%. Despite this progress, there is still limited knowledge on the fundamental photophysics. Here we use microwave photoconductance and photoluminescence measurements to investigate the temperature dependence of the carrier generation, mobility, and recombination in (CH3NH3)PbI3. At tem...

Journal: :Korean Journal of Metals and Materials 2022

Because of their superior optical, and electrical properties, lead halide perovskites have emerged as potential materials for light-emitting-diodes. However, some obstacles yet to be overcome practical applications including low exciton binding energy, the difficulty fabricating uniform perovskite films,, instability heat, light, moisture. In this review, we focus on strategies improve lifetime...

Journal: :ACS nano 2010
Carsten Georgi Alexander A Green Mark C Hersam Achim Hartschuh

We observe localization of excitons in semiconducting single-walled carbon nanotubes at room temperature using high-resolution near-field photoluminescence (PL) microscopy. Localization is the result of spatially confined exciton energy minima with depths of more than 15 meV connected to lateral energy gradients exceeding 2 meV/nm as evidenced by energy-resolved PL imaging. Simulations of excit...

2002
Raoul Kopelman

The experimental data on triplet exciton transport in isotopically mixed crystals of naphthalene/ perdeuteronaphthalene (paper I) are contrasted with singlet exciton transport in the same samples (20%-100%) and analyzed in terms of incoherent hopping models. The master equation approach is emphasized and extended. We modify the conventional continuum master equations via a physically plausible ...

Journal: :The Journal of chemical physics 2008
Kim Hyeon-Deuk Yoshitaka Tanimura Minhaeng Cho

We have calculated the nonlinear response function of a DNA duplex helix including the contributions from the exciton population and coherence transfers by developing an appropriate exciton theory as well as by utilizing a projector operator technique. As a representative example of DNA double helices, the B-form (dA)10-(dT)10 is considered in detail. The Green functions of the exciton populati...

2002
Seungwon Lee Jeongnim Kim Lars Jönsson John W. Wilkins Garnett W. Bryant Gerhard Klimeck

Many-body levels of optically excited and multiply charged InAs nanocrystals are studied with the semiempirical tight-binding model. Single-particle levels of unstrained spherical InAs nanocrystals are described by the spds* nearest-neighbor tight-binding model including spin-orbit coupling. For optically excited InAs nanocrystals, first-order corrections of electron-hole Coulomb and exchange i...

2012
David R. Yarkony Robert Silbey

The variational results for the free energy of an interacting exciton phonon system are used to derive expressions for the scattering rate and diffusion constant of an exciton in such a system. These expressions are applicable to both wide and narrow band cases, and includes the possibility of an abrupt transition from wide band (free) exciton to narrow band (localized) exciton. Some comments a...

Journal: :The Journal of chemical physics 2016
Sheikha Lardhi Dalal Noureldine Moussab Harb Ahmed Ziani Luigi Cavallo Kazuhiro Takanabe

Density functional theory calculation was conducted to determine the optoelectronic properties of bismuth titanate sillenite (Bi12TiO20) and perovskite-like (Bi4Ti3O12) structures. The lattice parameters were experimentally obtained from Rietveld analysis. The density functional perturbation theory approach was used with the standard Perdew-Burke-Ernzerhof functional and screened Coulomb hybrid...

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