نتایج جستجو برای: water splitting thermo
تعداد نتایج: 594230 فیلتر نتایج به سال:
From a conceptual standpoint, the water photoelectrolysis reaction is the simplest way to convert solar energy into fuel. It is widely believed that nanostructured photocatalysts can improve the efficiency of the process and lower the costs. Indeed, nanostructured light absorbers have several advantages over traditional materials. This includes shorter charge transport pathways and larger redox...
Charge transport in nanoparticle-based materials underlies many emerging energy-conversion technologies, yet assessing the impact of nanometre-scale structure on charge transport across micrometre-scale distances remains a challenge. Here we develop an approach for correlating the spatial distribution of crystalline and current-carrying domains in entire nanoparticle aggregates. We apply this a...
Hydrogen production by water splitting may be an appealing solution for future energy needs. To evolve hydrogen efficiently in a sustainable manner, it is necessary first to synthesize what we may call a 'super catalyst' for water oxidation, which is the more challenging half reaction of water splitting. An efficient system for water oxidation exists in the water oxidizing complex in cyanobacte...
Photochemical splitting of water into H2 and O2 using solar energy is a process of great economic and environmental interest. Since the discovery of the first water splitting system based on TiO2 and Pt in 1972 by Fujishima and Honda, over 130 inorganic materials have been discovered as catalysts for this reaction. This review discusses the known inorganic catalysts with a focus on structure–ac...
As the biological activation and oxidation of water takes place at an inorganic cluster of the stoichiometry CaMn4 O5 , manganese oxide is one of the materials of choice in the quest for versatile, earth-abundant water splitting catalysts. To probe basic concepts and aid the design of artificial water-splitting molecular catalysts, a hierarchical modeling strategy was employed that explores clu...
Based on first principles calculations, we predict semihydrogenated graphitic BN (sh-BN) sheet is a potential metal-free visible-light driven photocatalyst for water splitting. The ground state of sh-BN is a strip-like antiferromagnetic semiconductor with a band gap suitable for visible-light absorption. The redox potentials of water splitting are all located inside the band gap and the probabi...
Theoretical limiting efficiencies have a critical role in determining technological viability and expectations for device prototypes, as evidenced by the photovoltaics community's focus on detailed balance. However, due to their multicomponent nature, photoelectrochemical devices do not have an equivalent analogue to detailed balance, and reported theoretical efficiency limits vary depending on...
This paper presents a novice heuristic algorithm, Water Flow-like Algorithm (WFA), for solving discrete optimization problems, particularly the bin packing problems. WFA simulates solution agents as water flows traversing the terrain mapped from the objective function. Governed by the gravitation force, water flows from higher attitudes to lower ones. Driven by the fluid momentum, water flows a...
A series of heteroleptic strontium complexes (1-9) using a combination of different aminoalkoxides and 2,2,6,6-tetramethyl-3,5-heptanedionate (tmhd) were prepared to examine the effect of the bulkiness and coordination ability of the aminoalkoxide ligand in these complexes as well as potential strontium precursors. All complexes were characterized by FT-IR, FT-NMR, elemental analyses, and therm...
Zinc oxide nanowire photoanodes are chemically stabilized by conformal growth of an ultrathin shell of titania through atomic layer deposition, permitting their stable operation for water splitting in a strongly alkaline solution. Because of the passivation of zinc oxide surface charge traps by titania coating, core/shell nanowire arrays supply a photocurrent density of 0.5 mA/cm under simulate...
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