An estimate of tropospheric ozone concentrations was obtained from the difference in the Total Ozone Mapping Spectrometer (TOMS) data between the high Andes and the Pacific Ocean. From 1979 to 1992 the tropospheric ozone concentration apparently increased by 1.48 ± 0.40 percent per year or 0.21 ± 0.06 Dobson unit per year over South America and the surrounding oceans. An increase ...

Atmospheric Chemistry and Physics Discussions This discussion paper is/has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP if available. Abstract The decrease of the concentration of ozone depleting substances (ODS) in the stratosphere over the past decade raises the question to what extent observed changes in strat...

This paper summarises the validation of GOME total ozone retrieved using the Weighting Function Differential Optical Absorption Spectroscopy (WFDOAS) algorithm Version 1.0. This algorithm has been described in detail in a companion paper by Coldewey-Egbers et al. (2005). Compared to the operational GDP (GOME Data Processor) V3, several improvements to the total ozone retrieval have been introdu...

A method for assimilating observations of ozone was implemented in the three-dimensional global stratospheric chemistry transport model ROSE. The model contains an extensive photochemical scheme which includes heterogeneous chemistry and uses temperature and wind fields from the UKMO (United Kingdom Meteorological Office) stratospheric analysis. Ozone measurements obtained by the Microwave Limb...

The total ozone distribution in March 1997 showed very low values in the North Atlantic-European region, even lower than in the years before. A spatial pattern correlation between the zonally asymmetric part of total ozone and that of the 300 hPa surface geopotential of the Northern Hemisphere was applied to examine the spatial structure of the low ozone values and its dynamic dependence. A tre...

This study investigates anomalous ozone distributions over cloudy areas in Nimbus-7 (N7) and Earth-Probe (EP) TOMS version-7 data and analyzes the causes for ozone anomaly formation. A 5◦-longitude by 5◦-latitude region is defined to contain a Positive Ozone Anomaly (POA) or Negative Ozone Anomaly (NOA) if the correlation coefficient 5 between total ozone and reflectivity is ≥0.5 or ≤−0.5. The ...

Ozone concentrations have been decreasing globally for the last 20 years in part due to increasing chlorine concentrations in the stratosphere (WMO 1999). The most dramatic example of these reductions has been identified in the high latitude southern hemisphere, where ozone levels are nearly entirely depleted in the lower stratosphere during September and October each year. This phenomenon, whi...

This work describes the first method to determine the tropical tropospheric ozone column directly from the Total Ozone Mapping Spectrometer (TOMS) space-borne instrument based on the physical differences in ozonecolumn detection as a function of its scan-angle geometry. Comparisons to tropical ozonesonde observations suggest the accuracy of these retrievals is ;20%. Tropospheric ozone derived f...

Measurements of ozone, sensible heat, and latent heat fluxes and plant physiological parameters were made at a northern mixed hardwood forest located at the University of Michigan Biological Station in northern Michigan from June 27 to September 28, 2002. These measurements were used to calculate total ozone flux and partitioning between stomatal and non-stomatal sinks. Total ozone flux varied ...

This study evaluated hemato-histological changes of black porgy in recirculating aquaculture systems (RAS) with three different ozone doses (no ozone, 20 g, and 40 g ozone/kg feed day). During the 44-day study, black porgy did not show significant behavior changes or mortalities in both the ozonated systems displaying average total residual oxidants concentrations of 0.12 and 0.25 mg/L. There w...