The perovskite SrTiO3-LaAlO3 structure has advanced to a model system to investigate the rich electronic phenomena arising at polar oxide interfaces. Using first principles calculations and transport measurements we demonstrate that an additional SrTiO3 capping layer prevents atomic reconstruction at the LaAlO3 surface and triggers the electronic reconstruction at a significantly lower LaAlO3 f...

Epitaxial SrRuO3 thin films were grown on both (100) and (111) SrTiO3 substrates with atomically flat surfaces that are required to grow high-quality films of materials under debate. The following notable differences were observed in the (111)-oriented SrRuO3 films: (1) slightly different growth mode, (2) approximately 10 K higher ferromagnetic transition temperature, and (3) better conducting ...

Ferroelectric domain structures of epitaxial BiFeO3 thin films on miscut 001 SrTiO3 substrates have been studied by transmission electron microscopy. BiFeO3 on 0.8° miscut substrates are composed of both 109° and 71° domains; in contrast, only 71° stripe domains are observed in BiFeO3 on 4° miscut 001 SrTiO3 substrates. The domain width in BiFeO3 on 4° miscut substrates increases as film thickn...

We used infrared spectroscopic ellipsometry to investigate the electronic properties of LaTiO_{3}/SrTiO_{3} superlattices (SLs). Our results indicated that, independent of the SL periodicity and individual layer thickness, the SLs exhibited a Drude metallic response with sheet carrier density per interface approximately 3x10;{14} cm;{-2}. This is probably due to the leakage of d electrons at in...

To implement the complex brain functions of learning, forgetting and memory in a single electronic device is very advantageous for realizing artificial intelligence. As a proof of concept, memristive devices with a simple structure of Ni/Nb-SrTiO3/Ti were investigated in this work. The functions of learning, forgetting and memory were successfully mimicked using the memristive devices, and the ...

First-principles calculation was used to study the structural and electronic features of the low-dimensional oxide structure, SrTiO3/Sr1−xLaxTiO3 (x= 0.25) superlattices, constructed by submonolayer low-dimensional La doping into SrTiO3. We demonstrate a dimensionality crossover from three-dimensional (3D) to two-dimensional (2D) electronic behavior in the system. Two types of carriers, one con...

Using path-integral Monte Carlo simulations and an ab initio effective Hamiltonian, we study the effects of quantum fluctuations on structural phase transitions in the cubic perovskite compounds SrTiO3 and BaTiO3 . We find quantum fluctuations affect ferroelectric ~FE! transitions more strongly than antiferrodistortive ~AFD! ones, even though the effective mass of a single FE local mode is larg...

Thermoelectric energy conversion is widely recognized as a promising technology both for electric power generation in terms of waste heat recovery and for cooling of various electronic devices [1]. SrTiO3 based perovskites are among a number of candidate materials for such thermoelectric applications [2]. For the first time, we demonstrate the successful synthesis of (1-x)SrTiO3-xLa1/3NbO3 cera...

We grew SrTiO3 on SrTiO3(001) by pulsed laser deposition, using x-ray scattering to monitor the growth in real time. The time-resolved small-angle scattering exhibits a well-defined length scale associated with the spacing between unit-cell high surface features. This length scale imposes a discrete spectrum of Fourier components and rate constants upon the diffusion equation solution, evident ...

The discovery of two-dimensional electron gases (2DEGs) in SrTiO3-based heterostructures provides new opportunities for nanoelectronics. Herein, we create a new type of oxide 2DEG by the epitaxial-strain-induced polarization at an otherwise nonpolar perovskite-type interface of CaZrO3/SrTiO3. Remarkably, this heterointerface is atomically sharp and exhibits a high electron mobility exceeding 60...