The application of femtosecond pump-probe photoelectron spectroscopy to directly observe vibrational wave packets passing through an avoided crossing is investigated using quantum wave packet dynamics calculations. Transfer of the vibrational wave packet between diabatic electronic surfaces, bifurcation of the wave packet, and wave packet construction via nonadiabatic mixing are shown to be obs...

We describe traveling waves in a basic model for three-dimensional water-wave dynamics in the weakly nonlinear long-wave regime. Small solutions that are periodic in the direction of translation (or orthogonal to it) form an infinite-dimensional family. We characterize these solutions through spatial dynamics, by reducing a linearly ill-posed mixed-type initial-value problem to a center manifol...

We study numerically and experimentally self-focusing dynamics of femtosecond light pulses. By demonstrating the potential of three dimensional imaging technique for quantitative recovery of complex (arbitrarily shaped) wave packets, we monitor space-time transformation dynamics of 150-fs light pulse, which undergoes self-focusing and filamentation in water. Peculiar spatiotemporal and spectral...

The dynamics of vibrational wave packets excited in Na2 dimers in the triplet ground and excited states is investigated by means of helium nanodroplet isolation (HENDI) combined with femtosecond pump-probe spectroscopy. Different pathways in the employed resonant multiphoton ionization scheme are identified. Within the precision of the method, the wave packet dynamics appears to be unperturbed ...

Received October 2, 1992; revised manuscript received December 29, 1992 Separatrices and scaling laws in the switching dynamics of spatial solitary wave pixels are investigated. We show that the dynamics in the full model are similar to those in the plane-wave limit. Switching features may be indicated and explained by the motion of the (complex) solitary wave amplitude in the phase plane. We r...

Extreme surface waves in deep-water long-crested sea are often interpreted as a manifestation in real world of the so-called breathing solitons of the focusing nonlinear Schrödinger equation. While the spontaneous emergence of such coherent structures from nonlinear wave dynamics was demonstrated to take place in fiber optics systems, the same point remains far more controversial in the hydrody...

Extreme surface waves in a deep-water long-crested sea are often interpreted as a manifestation in the real world of the so-called breathing solitons of the focusing nonlinear Schrödinger equation. While the spontaneous emergence of such coherent structures from nonlinear wave dynamics was demonstrated to take place in fiber-optics systems, the same point remains far more controversial in the h...

The interactions between carriers and fields in semiconductors at low frequencies (<100 GHz) can be adequately described by numerical solution of the Boltzmann transport equation coupled with Poisson’s equation. As the frequency approaches the THz regime, the quasi-static approximation fails and full-wave dynamics must be considered. Here, we review recent advances in global modeling techniques...

The dynamics of vibrational wave packets excited in K2 dimers attached to superfluid helium nanodroplets is investigated by means of femtosecond pump-probe spectroscopy. The employed resonant three-photon-ionization scheme is studied in a wide wavelength range and different pathways leading to K 2 -formation are identified. While the wave packet dynamics of the electronic ground state is not in...