This paper presents data on the content of toxic elements (Mn, Ni, Zn, Cu, Pb, As, Cr, Cd and Co), technogenic (137Cs, 134Cs) natural radionuclides 238U 232Th series (234Th, 226Ra, 210Pb, 232Th) 40K in sediments collected from ten sampling stations along northern Bulgarian Black Sea coast for a period more than twenty years. Measurements were made by Gamma Spectrometry Inductively Coupled Plasm...