Atmospheric Chemistry and Physics Discussions This discussion paper is/has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP if available. Abstract In the present study, the impact of aerosols on the photochemistry in Mexico City is evaluated using the WRF-CHEM model for the period from 24 to 29 March during the MCMA-...

An aerosol optical depth (AOD) three-dimensional variational data assimilation technique is developed for the Gridpoint Statistical Interpolation (GSI) system for which WRF-Chem forecasts are performed with a detailed sectional model, the Model for Simulating Aerosol Interactions and Chemistry (MOSAIC). Within GSI, forward AOD and adjoint sensitivities are performed using Mie computations from ...

The configuration and evaluation of the meteorology is presented for simulations over the South Asian region using the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem). Temperature, water vapor, dew point temperature, zonal and meridional wind components, precipitation and tropopause pressure are evaluated against radiosonde and satellite-borne (AIRS and TRMM) observatio...

Deteriorating air quality is one of the major problems faced worldwide and in particular in Asia. The world's most polluted megacities are located in Asia highlighting the urgent need for efforts to improve the air quality. New Delhi (India), one of the world's most polluted cities, was the host of the Common Wealth Games during the period of 4-14 October 2010. This high profile event provided ...

The Weather Research and Forecasting model coupled with chemistry (WRF-Chem) is modified to include a volatility basis set (VBS) treatment of secondary organic aerosol formation. The VBS approach, coupled with SAPRC-99 gas-phase chemistry mechanism, is used to model gas-particle partitioning and multiple generations of gas-phase oxidation of organic vapors. In addition to the detailed 9-species...

The response of the Indian summer monsoon (ISM) circulation and precipitation to Middle East dust aerosols on sub-seasonal timescales is studied using observations and the Weather Research and Forecasting model coupled with online chemistry (WRF-Chem). Satellite data show that the ISM rainfall in coastal southwest India, central and northern India, and Pakistan is closely associated with the Mi...

The aim of this study was to evaluate the ability of Neutrophil Gelatinase-Associated Lipocalin (NGAL) to predict clinically relevant worsening renal function (WRF) in acute heart failure (AHF). Plasma NGAL and serum creatinine changes during the first 4 days of admission were investigated in 1447 patients hospitalized for AHF and enrolled in the Placebo-Controlled Randomized Study of the Selec...

The atmospheric transport and ground deposition of radioactive isotopes 131I and 137Cs during and after the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident (March 2011) are investigated using the Weather Research and Forecasting-Chemistry (WRF-Chem) model. The aim is to assess the skill of WRF in simulating these processes and the sensitivity of the model’s performance to various parame...

Atmospheric inversion typically relies on the specification of prior flux and atmospheric model transport errors, which have large uncertainties. Here, we used ACT-America airborne observations to compare observation mismatch in eastern U.S. during four climatological seasons for mesoscale WRF(-Chem) global scale CarbonTracker/TM5 (CT) models. Models identical surface carbon fluxes, CT was as b...