Fluorination of CNx Nanotubes

نویسندگان

  • A. V. Okotrub
  • N. Maksimova
  • T. A. Duda
  • A. G. Kudashov
  • Yu. V. Shubin
  • D. S. Su
  • E. M. Pazhetnov
  • A. I. Boronin
  • L. G. Bulusheva
چکیده

Multiwall CNx nanotubes have been prepared by thermal decomposition of acetonitrile over Co/Ni catalytic particles. The fluorination of nanotubes was performed at roomtemperature by using a gaseous mixture of BrF3 and Br2. Transmission electron microscopy (TEM) and x-ray diffraction (XRD) indicated that only the outer shells of CNx nanotubes were fluorinated, whereas the inner shells remained intact. Xray photoelectron spectroscopy (XPS) showed an oxidation of pyridinic-type nitrogenwith tube fluorination.

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تاریخ انتشار 2006